Roshan F. DSouza's profile
Journal Article

Polymaleimide-Based Polysulfobetaines Bearing Functional and Nonfunctional Hydrophobic Units and Its Aggregation Behavior in Aqueous Media

Langmuir · 2019
Dsouza, R.F., Parthiban, A.
3
Citations
2019
Published

Abstract

Copolymaleimide based zwitterionic polysulfobetaines (PM-SBs) were prepared by a "top down" method for the first time. Interfacial studies of these polymers showed many interesting characteristics. These PM-SBs did not require any salt in the form of sodium chloride (NaCl) to dissolve in water and exhibited exceptional salt tolerance. PM-SBs showed very mild thermogelling behaviour. The viscosity of 5 wt% aqueous solution of polymers increased with increasing concentration of salt without showing any limits within the salt concentrations studied [200g/L of NaCl (3.4 M)] in contrast to other reported zwitterionic polysulfobetaines. Dynamic light scattering (DLS) studies also indicated a structure dependent particle size with varying concentration of NaCl solution. The uniformity of particles of 5 wt% aqueous solution of PM-SBs increased with increasing concentration of NaCl. At 0.1 wt% concentration, even in the absence of NaCl, mild aggregation was noticed. The concentration of aggregated particles increased with the increasing concentration of NaCl. Because of the exceptionally high salt tolerance, these polymers are potentially suitable for applications in antifouling, oil field, personal care formulations and water purification.

Fields of Study

Aqueous solution Chemistry Bearing (navigation) Hydrophobic effect Chemical engineering Organic chemistry Computer science Engineering Biology Immunology